Erika Howsare at C-Ville has an interesting look at getting around Charlottesville without a car.
Very related article I wrote in 2006 – Are there Two Charlottesvilles?
Also: Patience Crabstick wrote earlier this year a detailed account of the Charlottesville Bus system. (and I wrote about her writing about the bus system)
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A good real estate agent can help you find neighborhoods in Charlottesville that are great for getting around on foot or using public transportation.